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Conversion of carbon dioxide in atmospheric pressure dielectric barrier discharges with different electrode configurations
Wang C(王超); Wang, HaiXing; Liu CY(刘昌裕); Meng X(孟显); Jin, GuangYuan; Huang HJ(黄河激); Cao JW(曹进文); Sun, SuRong; Yan C(闫聪)
Source PublicationPHYSICA SCRIPTA
2023-08-01
Volume98Issue:8Pages:85605
ISSN0031-8949
AbstractThe choice of electrode configuration and dielectric material is critical to the discharge process and plasma characteristics of a dielectric barrier discharge (DBD) reactor. In this study, a new electrode configuration of DBD reactor with copper mesh as electrode inserted between dielectrics is proposed, which has a much higher capacitance than the conventional double-dielectric layer DBD reactor. Two materials with different relative dielectric permittivities, alumina and zirconia, are chosen as dielectrics for an experimental comparison of CO2 decomposition. The experimental results show that the conversion rate of CO2 for the reactor with copper mesh inserted between dielectrics are higher than that of the corresponding double dielectric layer reactor under the same discharge power, and the conversion rate of CO2 with zirconia as a dielectric material is higher than the case of alumina as a dielectric. Further analysis of discharge characteristics shows that for the reactor with copper mesh inserted between dielectrics, the applied voltage required for discharge is significantly reduced, the amount of transferred charge is significantly increased, and the number of micro-discharge current pulses as well as the average lifetime during a single voltage cycle are also considerably increased, leading to an increase in the CO2 discharge efficiency and conversion rate.
Keywordcarbon dioxide decomposition DBD electrode configuration
DOI10.1088/1402-4896/ace2fe
Indexed BySCI ; EI
Language英语
WOS IDWOS:001028184500001
WOS Research AreaPhysics
WOS SubjectPhysics, Multidisciplinary
Funding OrganizationNational Natural Science Foundation of China [12175011, 12005010, 11735004] ; State Key Laboratory of High-temperature Gas Dynamics, Chinese Academy of Sciences [2021KF08]
Classification二类
Ranking1
ContributorWang, HX (corresponding author), Beihang Univ, Sch Astronaut, Beijing 102206, Peoples R China. ; Meng, X (corresponding author), Chinese Acad Sci, Inst Mech, Beijing 100190, Peoples R China. ; Wang, HX (corresponding author), Beihang Univ, Ningbo Inst Technol, Ningbo 315800, Peoples R China.
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Cited Times:1[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://dspace.imech.ac.cn/handle/311007/92562
Collection高温气体动力学国家重点实验室
宽域飞行工程科学与应用中心
Affiliation1.{Wang, Chao, Wang, Hai-Xing, Liu, Chang-Yu, Jin, Guang-Yuan, Sun, Su-Rong} Beihang Univ, Sch Astronaut, Beijing 102206, Peoples R China
2.{Wang, Chao, Liu, Chang-Yu, Meng, Xian, Huang, He-Ji, Cao, Jin-Wen, Yan, Cong} Chinese Acad Sci, Inst Mech, Beijing 100190, Peoples R China
3.{Wang, Hai-Xing, Sun, Su-Rong} Beihang Univ, Ningbo Inst Technol, Ningbo 315800, Peoples R China
Recommended Citation
GB/T 7714
Wang C,Wang, HaiXing,Liu CY,et al. Conversion of carbon dioxide in atmospheric pressure dielectric barrier discharges with different electrode configurations[J]. PHYSICA SCRIPTA,2023,98,8,:85605.Rp_Au:Wang, HX (corresponding author), Beihang Univ, Sch Astronaut, Beijing 102206, Peoples R China., Meng, X (corresponding author), Chinese Acad Sci, Inst Mech, Beijing 100190, Peoples R China., Wang, HX (corresponding author), Beihang Univ, Ningbo Inst Technol, Ningbo 315800, Peoples R China.
APA 王超.,Wang, HaiXing.,刘昌裕.,孟显.,Jin, GuangYuan.,...&闫聪.(2023).Conversion of carbon dioxide in atmospheric pressure dielectric barrier discharges with different electrode configurations.PHYSICA SCRIPTA,98(8),85605.
MLA 王超,et al."Conversion of carbon dioxide in atmospheric pressure dielectric barrier discharges with different electrode configurations".PHYSICA SCRIPTA 98.8(2023):85605.
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