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Toughening two dimensional materials through lattice disorder
Xie WH(谢文慧); Zhang XB(张曦蓓); Wei YJ(魏宇杰); Gao, Huajian
Corresponding AuthorWei, Yujie([email protected]) ; Gao, Huajian([email protected])
Source PublicationCARBON
2023-09-01
Volume213Pages:9
ISSN0008-6223
AbstractCarbon-based two-dimensional (2D) materials, with graphene being the most prominent example, are some of the strongest materials existing today due to their covalent bonding but at the same time also the most fragile, with fracture toughness close to that of an ideally brittle solid, due to their intrinsic lack of effective dissipation mechanisms. Here, by investigating fracture mechanisms in monolayer amorphous carbon (MAC), we reveal a novel strategy to toughen 2D materials through lattice disorder. It is shown that lattice disorder results in rippling which can alleviate stress concentration in the vicinity of crack-tips and render MAC flaw tolerant. Consequently, MAC outperforms graphene in resisting brittle fracture and endures larger strain to failure in the presence of a preexisting crack. Our work sheds light on the mechanisms of crack propagation in MAC and also suggests that it might be generally possible to design tough 2D materials through lattice disorder.
KeywordMonolayer amorphous carbon Lattice disorder Toughening Rippling Graphene
DOI10.1016/j.carbon.2023.118268
Indexed BySCI ; EI
Language英语
WOS IDWOS:001147674000001
WOS KeywordREACTIVE FORCE-FIELD ; MECHANICAL-PROPERTIES ; INTRINSIC STRENGTH ; SUSPENDED GRAPHENE ; ELASTIC PROPERTIES ; FRACTURE ; DEFECTS ; TOUGHNESS ; CARBON ; SIZE
WOS Research AreaChemistry ; Materials Science
WOS SubjectChemistry, Physical ; Materials Science, Multidisciplinary
Funding ProjectNSFC Basic Science Center Program for 'Multiscale Problems in Nonlinear Mechanics '[11988102] ; Nanyang Technological University[002479 -00001] ; Agency for Science, Technology and Research (A*STAR) in Singapore
Funding OrganizationNSFC Basic Science Center Program for 'Multiscale Problems in Nonlinear Mechanics ' ; Nanyang Technological University ; Agency for Science, Technology and Research (A*STAR) in Singapore
Classification一类
Ranking1
ContributorWei, Yujie ; Gao, Huajian
Citation statistics
Cited Times:8[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://dspace.imech.ac.cn/handle/311007/94250
Collection非线性力学国家重点实验室
Recommended Citation
GB/T 7714
Xie WH,Zhang XB,Wei YJ,et al. Toughening two dimensional materials through lattice disorder[J]. CARBON,2023,213:9.Rp_Au:Wei, Yujie, Gao, Huajian
APA 谢文慧,张曦蓓,魏宇杰,&Gao, Huajian.(2023).Toughening two dimensional materials through lattice disorder.CARBON,213,9.
MLA 谢文慧,et al."Toughening two dimensional materials through lattice disorder".CARBON 213(2023):9.
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