| Connection between Mechanical Relaxation and Equilibration Kinetics in a High-Entropy Metallic Glass | |
Duan, YJ1,2; Nabahat, M2; Tong, Yu3,4; OrtizMembrado, L5; JimenezPique, E5; Zhao K(赵坤)6,7; Wang YJ(王云江)6,7 ; Yang, Y8,9; Wada, T10; Kato, H10; Pellelier, JM11; Qiao, JC1; Pineda, E2
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| Corresponding Author | Qiao, J. C.([email protected]) ; Pineda, E.([email protected]) |
| Source Publication | PHYSICAL REVIEW LETTERS
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| 2024-01-29 | |
| Volume | 132Issue:5Pages:7 |
| ISSN | 0031-9007 |
| Abstract | The slow transition from an out-of-equilibrium glass towards a supercooled liquid is a complex relaxation phenomenon. In this Letter, we study the correlation between mechanical relaxation and equilibration kinetics in a Pd20Pt20Cu20Ni20P20 high-entropy metallic glass. The evolution of stress relaxation with aging time was obtained with an unprecedented detail, allowing us to pinpoint new interesting features. The long structural relaxation towards equilibrium contains a wide distribution of activation energies, instead of being just associated to the beta relaxation as commonly accepted. The stress relaxation time can be correlated with the equilibration rate and we observe a decrease of microstructural heterogeneity which contrasts with an increase of dynamic heterogeneity. These results significantly enhance our insight of the interplay between relaxation dynamics and thermodynamics in metallic glasses. |
| DOI | 10.1103/PhysRevLett.132.056101 |
| Indexed By | SCI ; EI |
| Language | 英语 |
| WOS ID | WOS:001181999900002 |
| WOS Keyword | BETA-RELAXATION ; SPATIAL HETEROGENEITY ; SECONDARY RELAXATION ; ELASTIC-MODULUS ; INDENTATION ; BEHAVIOR ; DYNAMICS ; REJUVENATION ; TRANSITION ; HARDNESS |
| WOS Research Area | Physics |
| WOS Subject | Physics, Multidisciplinary |
| Funding Project | NSFC[51971178] ; NSFC[52271153] ; NSFC[12072344] ; Natural Science Basic Research Plan for Distinguished Young Scholars in Shaanxi Province[2021JC-12] ; Fundamental Research Funds for the Central Universities[D5000220034] ; FY2023 GIMRT[202212-RDKGE-0504] ; Youth Innovation Promotion Association of the Chinese Academy of Sciences ; Research Grant Council (RGC) ; Hong Kong government through the General Research Fund (GRF)[CityU11206362] ; Hong Kong government through the General Research Fund (GRF)[CityU11201721] ; MCIN/AEI[PID2020-112975GB-I00] ; MCIN/AEI[PID2021-126614OB-I00] ; Generalitat de Catalunya ; AGAUR[2021SGR00343] ; Innovation Foundation for Doctor Dissertation of Northwestern Polytechnical University[CX202031] ; China Scholarship Council (CSC)[202006290092] |
| Funding Organization | NSFC ; Natural Science Basic Research Plan for Distinguished Young Scholars in Shaanxi Province ; Fundamental Research Funds for the Central Universities ; FY2023 GIMRT ; Youth Innovation Promotion Association of the Chinese Academy of Sciences ; Research Grant Council (RGC) ; Hong Kong government through the General Research Fund (GRF) ; MCIN/AEI ; Generalitat de Catalunya ; AGAUR ; Innovation Foundation for Doctor Dissertation of Northwestern Polytechnical University ; China Scholarship Council (CSC) |
| Classification | 一类 |
| Ranking | 3+ |
| Contributor | Qiao, J. C. ; Pineda, E. |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://dspace.imech.ac.cn/handle/311007/94882 |
| Collection | 非线性力学国家重点实验室 |
| Affiliation | 1.Northwestern Polytech Univ, Sch Mech Civil Engn & Architecture, Xian 710072, Peoples R China; 2.Univ Politecn Cataluna, Inst Energy Technol, Dept Phys, Barcelona 08019, Spain; 3.Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, CAS Key Lab Magnet Mat & Devices, Ningbo 315201, Peoples R China; 4.Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Zhejiang Prov Key Lab Magnet Mat & Applicat Techno, Ningbo 315201, Peoples R China; 5.Univ Politecn Cataluna, Dept Mat Sci, Barcelona 08019, Spain; 6.Chinese Acad Sci, Inst Mech, State Key Lab Nonlinear Mech, Beijing 100190, Peoples R China; 7.Univ Chinese Acad Sci, Sch Engn Sci, Beijing 100049, Peoples R China; 8.City Univ Hong Kong, Coll Engn, Dept Mech Engn, Tat Chee Ave,Kowloon Tong, Hong Kong, Peoples R China; 9.City Univ Hong Kong, Coll Engn, Dept Mat Sci & Engn, Tat Chee Ave,Kowloon Tong, Hong Kong, Peoples R China; 10.Tohoku Univ, Inst Mat Res, Sendai 9808577, Japan; 11.Univ Lyon, MATEIS, CNRS, UMR 5510,INSA Lyon, Batiment Blaise Pascal, F-69621 Lyon, France |
| Recommended Citation GB/T 7714 | Duan, YJ,Nabahat, M,Tong, Yu,et al. Connection between Mechanical Relaxation and Equilibration Kinetics in a High-Entropy Metallic Glass[J]. PHYSICAL REVIEW LETTERS,2024,132,5,:7.Rp_Au:Qiao, J. C., Pineda, E. |
| APA | Duan, YJ.,Nabahat, M.,Tong, Yu.,OrtizMembrado, L.,JimenezPique, E.,...&Pineda, E.(2024).Connection between Mechanical Relaxation and Equilibration Kinetics in a High-Entropy Metallic Glass.PHYSICAL REVIEW LETTERS,132(5),7. |
| MLA | Duan, YJ,et al."Connection between Mechanical Relaxation and Equilibration Kinetics in a High-Entropy Metallic Glass".PHYSICAL REVIEW LETTERS 132.5(2024):7. |
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