Manipulation of Contact Angle Hysteresis at Electrified Ionic Liquid-Solid Interfaces | |
Nie PC(聂鹏程)1,2; Jiang XK(蒋玺恺)1; Zheng X(郑旭)1; Guan DS(关东石)1,2 | |
Corresponding Author | Guan, Dongshi([email protected]) |
Source Publication | PHYSICAL REVIEW LETTERS
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2024-01-25 | |
Volume | 132Issue:4Pages:6 |
ISSN | 0031-9007 |
Abstract | Room-temperature ionic liquids (RTILs) are intriguing fluids that have drawn much attention in applications ranging from tribology and catalysis to energy storage. With strong electrostatic interaction between ions, their interfacial behaviors can be modulated by controlling energetics of the electrified interface. In this work, we report atomic-force-microscope measurements of contact angle hysteresis (CAH) of a circular contact line formed on a micron-sized fiber, which is coated with a thin layer of conductive film and intersects an RTIL-air interface. The measured CAH shows a distinct change by increasing the voltage U applied on the fiber surface. Molecular dynamics simulations were performed to illustrate variations of the solidlike layer in the RTIL adsorbed at the electrified interface. The integrated experiments and computations demonstrate a new mechanism to manipulate the CAH by rearrangement of interfacial layers of RTILs induced by the surface energetics. |
DOI | 10.1103/PhysRevLett.132.044002 |
Indexed By | SCI ; EI |
Language | 英语 |
WOS ID | WOS:001182014200010 |
WOS Keyword | PERIODIC SLAB GEOMETRIES ; ELECTROSTATICS ; SOLVENTS |
WOS Research Area | Physics |
WOS Subject | Physics, Multidisciplinary |
Funding Project | NSFC[11972351] ; NSFC Basic Science Center Program for Multiscale Problems in Nonlinear Mechanics[11988102] ; Chinese Academy of Sciences[025GJHZ2022023MI] |
Funding Organization | NSFC ; NSFC Basic Science Center Program for Multiscale Problems in Nonlinear Mechanics ; Chinese Academy of Sciences |
Classification | 一类 |
Ranking | 1 |
Contributor | Guan, Dongshi |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://dspace.imech.ac.cn/handle/311007/94912 |
Collection | 非线性力学国家重点实验室 |
Affiliation | 1.Chinese Acad Sci, Inst Mech, State Key Lab Nonlinear Mech, Beijing 100080, Peoples R China; 2.Univ Chinese Acad Sci, Sch Engn Sci, Beijing 100049, Peoples R China |
Recommended Citation GB/T 7714 | Nie PC,Jiang XK,Zheng X,et al. Manipulation of Contact Angle Hysteresis at Electrified Ionic Liquid-Solid Interfaces[J]. PHYSICAL REVIEW LETTERS,2024,132,4,:6.Rp_Au:Guan, Dongshi |
APA | 聂鹏程,蒋玺恺,郑旭,&关东石.(2024).Manipulation of Contact Angle Hysteresis at Electrified Ionic Liquid-Solid Interfaces.PHYSICAL REVIEW LETTERS,132(4),6. |
MLA | 聂鹏程,et al."Manipulation of Contact Angle Hysteresis at Electrified Ionic Liquid-Solid Interfaces".PHYSICAL REVIEW LETTERS 132.4(2024):6. |
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