| Strain Engineering of Ion-Coordinated Nanochannels in Nanocellulose | |
| Li, JiaHao; Hou, YuanZhen; He, ZeZhou; Wu HA(吴恒安); Zhu, YinBo | |
| Corresponding Author | Zhu, YinBo([email protected]) |
| Source Publication | NANO LETTERS
 |
| 2024-05-14 | |
| Volume | 24Issue:21Pages:6262-6268 |
| ISSN | 1530-6984 |
| Abstract | Expanding the interlayer spacing plays a significant role in improving the conductivity of a cellulose-based conductor. However, it remains a challenge to regulate the cellulose nanochannel expanded by ion coordination. Herein, starting from multiscale mechanics, we proposed a strain engineering method to regulate the interlayer spacing of the cellulose nanochannels. First-principles calculations were conducted to select the most suitable ions for coordination. Large-scale molecular dynamics simulations were performed to reveal the mechanism of interlayer spacing expansion by the ion cross-linking. Combining the shear-lag model, we established the relationship between interfacial cross-link density and interlayer spacing of an ion-coordinated cellulose nanochannel. Consequently, fast ion transport and current regulation were realized via the strain engineering of nanochannels, which provides a promising strategy for the current regulation of a cellulose-based conductor. |
| Keyword | nanocellulose cellulose nanochannel ion transport strain engineering ion cross-linking |
| DOI | 10.1021/acs.nanolett.4c00867 |
| Indexed By | SCI ; EI |
| Language | 英语 |
| WOS ID | WOS:001225234300001 |
| WOS Keyword | LENGTH SCALES ; CROSS-LINKING ; GRAPHENE ; LOCALIZATION ; COMPOSITES ; BATTERIES |
| WOS Research Area | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
| WOS Subject | Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter |
| Funding Project | National Natural Science Foundation of China[2022465] ; Youth Innovation Promotion Association CAS[12232016] ; Youth Innovation Promotion Association CAS[12172346] ; Youth Innovation Promotion Association CAS[12202431] ; National Natural Science Foundation of China[2208085QA24] ; Natural Science Foundation of Anhui Province ; Supercomputing Center of University of Science and Technology of China |
| Funding Organization | National Natural Science Foundation of China ; Youth Innovation Promotion Association CAS ; National Natural Science Foundation of China ; Natural Science Foundation of Anhui Province ; Supercomputing Center of University of Science and Technology of China |
| Classification | 一类 |
| Ranking | 3+ |
| Contributor | Zhu, YinBo |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://dspace.imech.ac.cn/handle/311007/95364 |
| Collection | 非线性力学国家重点实验室 |
| Recommended Citation GB/T 7714 | Li, JiaHao,Hou, YuanZhen,He, ZeZhou,et al. Strain Engineering of Ion-Coordinated Nanochannels in Nanocellulose[J]. NANO LETTERS,2024,24,21,:6262-6268.Rp_Au:Zhu, YinBo |
| APA | Li, JiaHao,Hou, YuanZhen,He, ZeZhou,吴恒安,&Zhu, YinBo.(2024).Strain Engineering of Ion-Coordinated Nanochannels in Nanocellulose.NANO LETTERS,24(21),6262-6268. |
| MLA | Li, JiaHao,et al."Strain Engineering of Ion-Coordinated Nanochannels in Nanocellulose".NANO LETTERS 24.21(2024):6262-6268. |
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